- Laurence Harvey
- Wilhelm Grimm / The Cobbler (segment "The Cobbler and the Elves")
- Karlheinz Böhm
- Jacob Grimm
- Claire Bloom
- Dorothea Grimm
- Walter Slezak
- Stossel
- Barbara Eden
- Greta Heinrich
- Oscar Homolka
- The Duke
- Arnold Stang
- Rumpelstiltskin
- Martita Hunt
- Anna Richter
- Betty Garde
- Miss Bettenhausen
- Bryan Russell
- Friedrich Grimm
- Ian Wolfe
- Gruber
- Tammy Marihugh
- Pauline Grimm
- Cheerio Meredith
- Mrs. Von Dittersdorf
- Walter Rilla
- Priest
- Yvette Mimieux
- The Princess (segment "The Dancing Princess")
- Russ Tamblyn
- The Woodsman (segment "The Dancing Princess")
- Jim Backus
- The King (segment "The Dancing Princess")
- Beulah Bondi
- The Gypsy (segment "The Dancing Princess")
- Clinton Sundberg
- The Prime Minister (segment "The Dancing Princess")
- Walter Brooke
- The Mayor (segment "The Cobbler and the Elves")
- Sandra Bettin
- The Ballerina (segment "The Cobbler and the Elves")
- Robert Foulk
- The Hunter (segment "The Cobbler and the Elves")
- Terry-Thomas
- Ludwig (segment "The Singing Bone")
- Buddy Hackett
- Hans (segment "The Singing Bone")
- Otto Kruger
- The King (segment "The Singing Bone")
- Robert Crawford Jr.
- The Shepherd (segment "The Singing Bone")
- Sydney Smith
- The Spokesman (segment "The Singing Bone")
- Pamela Baird
- Cinderella
- Billy Barty
- The Court Jester (segment "The Dancing Princess")
- Jeanine Cashell
- Princess Aide (segment "The Dancing Princess")
- Regensburger Domspatzen
- Children Choir in Rheinburg
- Diana Driscoll
- Gretel
- True Ellison
- Snow White
- Stanley Fafara
- Hansel
- Darby Hinton
- Little Boy (segment "The Cobbler and the Elves")
- Eduard Linkers
- Painter
- Jon Lormer
- The Doctor
- Gregory Morton
- Dantino
- Elisabeth Neumann-Viertel
- Flower Vendor
- 'Little Billy' Rhodes
- Grumpy the Dwarf
- Ruthie Robinson
- Little Red Riding Hood
- Angelo Rossitto
- Dwarf
- Gene Roth
- Berlin Royal Academy Representative at Train Station
- Les Tremayne
- Prologue Narrator
- Peter Whitney
- The Giant
